A new carbon isotope record for two high-latitude sedimentary successions that span the Jurassic-Cretaceous boundary interval in the Sverdrup Basin of Arctic Canada is presented. This study, combined with other published Arctic data, shows a large negative isotopic excursion of organic carbon (δ¹³C_org) of 4‰ (V-PDB) and to a minimum of-30.7‰ in the probable middle Volgian Stage. This is followed by a return to less negative values of c.-27‰. A smaller positive excursion in the Valanginian Stage of c. 2‰, reaching maximum values of-24.6‰, is related to the Weissert Event. The Volgian isotopic trends are consistent with other high-latitude records but do not appear in δ¹³C_carb records of Tethyan Tithonian strata. In the absence of any obvious definitive cause for the depleted δ¹³C_org anomaly, we suggest several possible contributing factors. The Sverdrup Basin and other Arctic areas may have experienced compositional evolution away from open-marine δ¹³C values during the Volgian Age due to low global or large-scale regional sea levels, and later become effectively coupled to global oceans by Valanginian time when sea level rose. A geologically sudden increase in volcanism may have caused the large negative δ¹³C_org values seen in the Arctic Volgian records but the lack of precise geochronological age control for the Jurassic-Cretaceous boundary precludes direct comparison with potentially coincident events, such as the Shatsky Rise. This study offers improved correlation constraints and a refined C-isotope curve for the Boreal region throughout latest Jurassic and earliest Cretaceous time.