The well-preserved exposures of pillow basalts from the late Archean (2.7 Ga) Chitradurga greenstone belt (Western Dharwar Craton) have been studied in detail using petrological, bulk-rock geochemical and isotope data. The pillows are compositionally basalts to basaltic andesites, and constituted of actinolite and plagioclase. The pillows show slight to moderately depleted LREE (La/Sm_N = 0.6−1.03), and nearly flat HREE patterns (Gd/Yb_N = 1.03−1.17) that are comparable with MORBs, but have an overall depletion in REEs relative to the latter. The trace-element patterns of the pillows on an N-MORB normalized multi-element diagram, however, are broadly comparable with that of Island Arc Basalts. The pillows were perhaps generated during the initiation of an intra-oceanic subduction zone where a depleted upper mantle (MORB-source) was metasomatized with slab-derived aqueous fluids. The pillows show a whole-rock Sm–Nd errorchron age of 2433 ± 400 Ma, which is within error of the previously reported Sm–Nd age of 2747 ± 15 Ma. The Pb–Pb isochron age (2627 ± 82 Ma) of the pillows is much closer to the previously reported Sm–Nd age, and it may also indicate the 2.62 Ga thermal event associated with felsic magmatism in the Western Dharwar Craton.