Mapping spatial and temporal variation of seafloor organic matter Delta C-14 and delta C-13 in the Northern Gulf of Mexico following the Deepwater Horizon Oil Spill
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Mapping spatial and temporal variation of seafloor organic matter Delta C-14 and delta C-13 in the Northern Gulf of Mexico following the Deepwater Horizon Oil Spill. / Rogers, Kelsey L.; Bosman, Samantha H.; Wildermann, Natalie; Rosenheim, Brad E.; Montoya, Joseph P.; Hollander, David; Zhao, Tingting; Chanton, Jeffrey P.
I: Marine Pollution Bulletin, Bind 164, 112076, 2021.Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt
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T1 - Mapping spatial and temporal variation of seafloor organic matter Delta C-14 and delta C-13 in the Northern Gulf of Mexico following the Deepwater Horizon Oil Spill
AU - Rogers, Kelsey L.
AU - Bosman, Samantha H.
AU - Wildermann, Natalie
AU - Rosenheim, Brad E.
AU - Montoya, Joseph P.
AU - Hollander, David
AU - Zhao, Tingting
AU - Chanton, Jeffrey P.
PY - 2021
Y1 - 2021
N2 - Following the Deepwater Horizon oil spill of 2010, large amounts of biodegraded oil (petrocarbon) sank to the seafloor. Our objectives were to 1) determine post-spill isotopic values as the sediments approached a new baseline and 2) track the recovery of affected sediments. Sediment organic carbon Delta C-13 and Delta C-14 reached a post spill baseline averaging -21.2 +/- 0.9 parts per thousand (n = 129) and-220 +/- 66 parts per thousand (n = 95). Spatial variations in seafloor organic carbon baseline isotopic values, C-13 and C-14, were influenced by river discharge and hydrocarbon seepage, respectively. Inverse Distance Weighting of surface sediment Delta C-14 values away from seep sites showed a 50% decrease in the total mass of petrocarbon, from 2010 to 2014. We estimated a rate of loss of -2 x 10(9) g of petrocarbon-C/year, 2-11% of the degradation rates in surface slicks. Despite the observed recovery in sediments, lingering residual material in the surface sediments was evident seven years following the blowout.
AB - Following the Deepwater Horizon oil spill of 2010, large amounts of biodegraded oil (petrocarbon) sank to the seafloor. Our objectives were to 1) determine post-spill isotopic values as the sediments approached a new baseline and 2) track the recovery of affected sediments. Sediment organic carbon Delta C-13 and Delta C-14 reached a post spill baseline averaging -21.2 +/- 0.9 parts per thousand (n = 129) and-220 +/- 66 parts per thousand (n = 95). Spatial variations in seafloor organic carbon baseline isotopic values, C-13 and C-14, were influenced by river discharge and hydrocarbon seepage, respectively. Inverse Distance Weighting of surface sediment Delta C-14 values away from seep sites showed a 50% decrease in the total mass of petrocarbon, from 2010 to 2014. We estimated a rate of loss of -2 x 10(9) g of petrocarbon-C/year, 2-11% of the degradation rates in surface slicks. Despite the observed recovery in sediments, lingering residual material in the surface sediments was evident seven years following the blowout.
KW - Deepwater Horizon
KW - Radiocarbon
KW - Sediments
KW - Gulf of Mexico
KW - Carbon isotopes
KW - Petrocarbon
U2 - 10.1016/j.marpolbul.2021.112076
DO - 10.1016/j.marpolbul.2021.112076
M3 - Journal article
C2 - 33529879
VL - 164
JO - Marine Pollution Bulletin
JF - Marine Pollution Bulletin
SN - 0025-326X
M1 - 112076
ER -
ID: 260031416